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Skype for Business Mobile App + Smart Card Required
I'm using Skype for Business via my Office365 subscription and my domain in Office365 is federated against my on-prem ADFS-infrastructure. My user in the local AD have the option "Require Smart Card ...
MA will not help in this case has the Skype Business Mobile app will still require to enter a username and password.
Unfortunately, the scenario you describe is probably not supported.
The mobile client was not design to support Smart-Card.
JP